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[14] • • Business It's the birthday of soprano Jenny https://caleinang88.files.wordpress.com/2020/05/e-boek-pdf-wwpngxraua-5246.pdf https://www.commonsensemedia.org/book-reviews/one-crazy-summer https://www.e-learningforkids.org/ https://www.khanacademy.org/partner-content/big-history-project/solar-system-and-earth/knowing-solar-system-earth/v/bhp-intro-to-geology This study proposes the detn. of the electronic delocalization contribution to the Anomeric Effect (EDCAE, ΔΔEdeloc, eq 3) as a computational alternative in the evaluation of the excess of the axial preference shown by an electroneg. substituent located at α position to the annular heteroatom of a heterocyclic compd. (anomeric position) in both the presence and the absence of electronic delocalization retaining the same mol. geometry. The detn. of the EDCAE is computationally accessible through the application of the natural bond orbital anal. (NBO). 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Applying this methol. to cyclic and acyclic mols. at B3LYP/6-31G(d,p) and HF/6-31G(d,p)//B3LYP/6-31G(d,p) levels of theory, the anomeric effect shown by Cl in 1,3-dioxane; F, Cl, SMe, PH3, and CO2Me groups in 1,3-dithiane is of stereoelectronic nature while the preference of F, OMe, and NH2 in 1,3-dioxane and the P(O)Me2 group in 1,3-dithiane is not. also, this methodol. shows that anomeric effects without stereoelectronic origin can modify the mol. geometry in agreement with the geometric pattern required by the double-bond no-bond model, as recently proposed by Perrin.


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